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Structure-induced features of transport processes in an electroconsolidated FeNi composite

G. Ya. Khadzhai

V. N. Karazin Kharkiv National University, 4 Svobody Sq., Kharkiv 61022, Ukraine

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S. R. Vovk

V. N. Karazin Kharkiv National University, 4 Svobody Sq., Kharkiv 61022, Ukraine

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R. V. Vovk

V. N. Karazin Kharkiv National University, 4 Svobody Sq., Kharkiv 61022, Ukraine

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E. S. Gevorkyan

Ukrainian State University of Railway Transport, 7 Feierbakh Sq., Kharkiv 61050, Ukraine

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M. V. Kislitsa

V. N. Karazin Kharkiv National University, 4 Svobody Sq., Kharkiv 61022, Ukraine

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S. V. Dukarov

V. N. Karazin Kharkiv National University, 4 Svobody Sq., Kharkiv 61022, Ukraine

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S. I. Petrushenko

V. N. Karazin Kharkiv National University, 4 Svobody Sq., Kharkiv 61022, Ukraine

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A. Feher

Faculty of Science, P. J. Safarik University, Park Angelinum 9, 041 54 Kosice, Slovakia

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, and

O. V. Dobrovolskiy

https://orcid.org/0000-0002-7895-8265

Faculty of Physics, University of Vienna, Boltzmanngasse 5, 1090 Vienna, Austria

E-mail Address: [email protected]

Corresponding author.

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https://doi.org/10.1142/S021798492150425XCited by:0 (Source: Crossref)

Abstract

The structure and processes of mass, charge and heat transfer are investigated in an equiatomic Fe–Ni composite fabricated by electroconsolidation using the spark plasma sintering (SPS) technology. The system contains regions of almost pure Fe and Ni, separated by areas with variable concentration of components, formed in consequence of the interdiffusion in the electroconsolidation process. The interdiffusion coefficient of the Fe–Ni system has been revealed to be significantly higher than that of an alloy of a similar composition at the same temperature, which is likely the result of the employed SPS technology and the enhanced diffusion along the grain boundaries. The concentration dependence of the interdiffusion coefficient passes through a maximum at a Ni concentration of $\sim$ 70 at.%. The electrical and thermal conductivity of the studied system is significantly higher than that of an alloy of the same composition. The temperature dependence of the resistivity of the sample in the range 5–300 K is due to the scattering of electrons by defects and phonons, and the scattering of electrons by phonons fits well to the Bloch–Grüneisen–Wilson relation. The boundaries of the conductivity of the investigated composite correspond to the Hashin–Shtrikman boundaries for a three-phase system, if Fe, Ni and the FeNi alloy are selected as phases.

Keywords:

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Vol. 35, No. 24

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History

Received 20 May 2021

Revised 21 June 2021

Accepted 22 June 2021

Published: 30 July 2021

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Structure-induced features of transport processes in an electroconsolidated FeNi composite

Abstract

References

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Structure-induced features of transport processes in an electroconsolidated FeNi composite

Abstract

References

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