For the treatment of dye wastewater, it is of great significance to develop new adsorbents with high adsorption capacity and good separation effect. In this study, the Fe-Co magnetic activated carbon material (CN-Fe-Co-AC) was first prepared by high-temperature calcination. CN-Fe-Co-AC is physically characterized by various methods. CN-Fe-Co-AC can efficiently and quickly remove the organic dyes methylene blue (MB) and acid blue 80 (AB80). The adsorption of MB and acid blue based on CN-Fe-Co-AC adsorbent is mainly through the specific surface area and the functional groups on the surface. During this recovery process, the adsorption activity of CN-Fe-Co-AC for MB and AB80 decreased slightly. Kinetic data can be described using a Pseudo-second-order model and the data for adsorption equilibrium can be described using the Langmuir isotherm. The theoretical adsorption capacities of MB and AB80 are 104.82mg/g and 26.94mg/g, respectively. After repeated use of five times, the removal rate of MB exceeded 96%, and the removal rate of AB80 exceeded 75%. The excellent adsorption performance and recyclability of CN-Fe-Co-AC indicate that this material has certain potential application value.