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A method has been proposed to reason the choice among the known optimized models for methods for estimating chlorophyll (Chl) concentration in the seawater according to the information-logarithmic criterion, which provides a comparison of theoretical models by the SeaWiFS data. It has been shown that the most appropriate means is to determine the Chl concentration, since the concentration of Chl in seawater is systematically investigated by marine ships or remote sensing. All optimized models of the optical properties of seawater can be verified by checking the simulated and measured Chl concentration data.